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Magnetic dynamics of two-dimensional itinerant ferromagnet Fe3GeTe2
Among the layered two-dimensional ferromagnetic materials (2D FMs), due to a relatively high TC, the van der Waals (vdW) Fe3GeTe2 (FGT) crystal is of great importance for investigating its distinct magnetic properties. Recent, in collaboration with Prof Yongbing Xu’s group in School of Electronic Science and Engineering, Nanjing University, we published a work entitled “Magnetic dynamics of two-dimensional itinerant ferromagnet Fe3GeTe2” in Chin. Phys. B [Chin. Phys. B 30(9), 097501(2021)]. Congratulations to Ms. Lijun Ni. In this work, Here, we have carried out static and dynamic magnetization measurements of the FGT crystal with a Curie temperature Tc = 204 K.The M–H hysteresis loops with in-plane and out-of-plane orientations show that FGT has a strong perpendicular magnetic anisotropy with the easy axis along its c-axis. Moreover, we have calculated the uniaxial magnetic anisotropy constant (K1) from the SQUID measurements. The dynamic magnetic properties of FGT have been probed by utilizing the high sensitivity electron-spin-resonance (ESR) spectrometer at cryogenic temperatures. Based on an approximation of single magnetic domain mode, the K1 and the effective damping constant have also been determined from the out-of-plane angular dependence of ferromagnetic resonance (FMR) spectra obtained at the temperature range of 185 K to TC. We have found large magnetic damping with the effective damping constant ~ 0.58 along with a broad linewidth (delta H_pp > 1000 Oe at 9.48 GHz, H// c-axis). Our results provide useful dynamics information for the development of FGT-based spintronic devices.
Temperature and electric field effects on the dynamic modes in a spin current auto-oscillator
Our new work entitled ”Temperature and electric field effects on dynamic modes in spin current auto-oscillator”is published in Phys. Rev. B. [Phys. Rev. B 103, 144426(2021)]. In this work, we systematically study spectral characteristics of emission microwave signal by a spin current nano-oscillator (SCNO) based on TaOx/Py(3)/Pt(2) trilayers as a function of current, in-plane magnetic field angle, electrostatic gating, and temperature. The current dependence of spectral characteristics shows that such SCNO exhibits a single coherent oscillation mode at low currents, and then transfers into a multimode coexistence regime with several oscillation peaks, related to spatially separated oscillation regions, at high currents. The linewidth of these modes shows an exponential temperature dependence, indicating thermally activated mode transitions or mode hopping behavior among these spatially separated oscillation regions due to the mode coupling caused by strong thermal-magnon-mediated scattering rate at high temperatures. Additionally, electrostatic gating on oscillation frequency shows a temperature-independent behavior, but gets enhanced in the strongly nonlinear oscillation regime. The enhanced phenomenon is caused by a combination of nonlinear frequency redshift and driving current shift due to electric-field modulation of current-induced spin-orbit torques. The demonstrated electric-field and current control of three-terminal SCNO provides an efficient approach to developing electrically tunable microwave generators in radio frequency integrated circuits and spin-wave-based logic gates in magnonic devices.
Controllable excitation of multiple spin wave bullet modes in a spin Hall nano-oscillator based on [Ni/Co]/Pt multilayers
Spin-torque nano-oscillators are promising candidates for many radio frequency and magnon-based nanodevices due to their broad frequency tunability, easy fabrication and high durability. Our new work entitled ”Controllable excitation of multiple spin wave bullet modes in a spin Hall nano-oscillator based on [Ni/Co]/Pt multilayers” is published in Nanoscale [Nanoscale, 13, 7838-7843(2021)]. To explore the tunability, in this work, we chose a [Ni/Co]/Pt-based spin Hall nano-oscillator with a moderate uniaxial anisotropy to systematically study the corresponding magnetodynamics excited by locally injecting a dc current into a nanoscale region of the extended multilayers [Ni/Co]/Pt under certain conditions. We find that the excitation current, the magnitude and orientation of magnetic field, and temperature can be used as a tool to selectively excite certain frequency bullet modes. The transition between nonlinear self-localized bullet modes with different frequencies is caused by the experimental parameter-induced change of energy landscape because, in the [Ni/Co]/Pt system, the strong spatial fluctuation of interfacial magnetic anisotropy leads to the variations of the internal magnetic field of the actual device. Our results demonstrate that the fluctuations of magnetic properties can promote experimental control of spin-torque driven magnetization dynamics in spin Hall nano-oscillators, and the application of expediting nonlinear magnetization oscillators in magnon-based devices and neuromorphic computing.
Collimated Bidirectional Propagating Spin Wave Generated by a Nonlocal Spin-Current Nano-oscillator
Pure spin currents, generated by nonlocal spin injection and spin-orbit effects, have been widely used to control magnetization reversal and dynamics by current without charge transfer and its side effects in the device’s actual working region. Our new work entitled”Collimated Bidirectional Propagating Spin Wave Generated by a Nonlocal Spin-Current Nano-oscillator” is published in Phys. Rev. Applied [Phys. Rev. Applied 16, 034044(2021)]. Congratulations to Dr. Lina Chen and Mr. Zhenyu Gao. In this work, we experimentally demonstrate that a single coherent spin-wave mode can be excited by the pure spin current in a nonlocal spin-injection spin-valve device. The microwave spectra show that the observed spin-wave frequency is higher than the ferromagnetic resonance frequency, and almost does not change with the excitation current at moderate magnetic fields, indicating that the observed dynamical mode is a linear propagating spin-wave mode. Furthermore, micromagnetic simulations based on our device geometry generally reproduce the experimentally observed field-dependent and current-dependent oscillation characteristics, and provide us with the additional spatial information that the spin-wave mode exhibits collimated and bidirectional propagation paths in the direction perpendicular to the applied magnetic field. Our simulation results also show that the current local Oersted field in our nonlocal device is much smaller than in conventional nanocontact magnetic oscillators, and has a minimal impact on the spin-wave dynamics. A near-symmetrically-collimated and bidirectional propagating spin-wave beam with magnetic field–controllable beam direction and current-dependent frequency, achieved in our demonstrated nonlocal spin-current nano-oscillator, can be used as a local spin-wave source for magnonic logic devices and can be used to build daisy-chaining oscillatory neural networks with mutual synchronization.
Observation of topological Hall effect in antiferromagnetic FeRh film
In collaboration with Prof. Dunhui Wang’s group in our physical department, we published a paper entitled “Observation of topological Hall effect in antiferromagnetic FeRh film”in APL [Applied Physical Letters 115, 022404 (2019)]. Noncollinear magnetic structures can give rise to peculiar Hall effects and hold promise for next-generation spintronic devices. In this work, we report the observation of the topological Hall effect (THE) through electrical transport measurements in antiferromagnetic B2-ordered FeRh thin films grown by sputtering techniques on a MgO (001) substrate. Our results opens the possibility to discover the topological Hall effect in centrosymmetric antiferromagnets in contrast to the widely reported B20-type chiral magnets.
New progress in the dynamical mode coupling and coherence in a nano-oscillator
Controlling dynamical mode coupling in magnetic nano-oscillators is essential to improving their microwave spectral properties for rf applications and neuromorphic computing. Progress here is held back by the lack of a suitable platform that provides controlled coupling. This study experimentally demonstrates control of dynamical mode coupling in spin Hall nano-oscillators with perpendicular magnetic anisotropy, by means of temperature, excitation current, and magnetic field. It is established that mode coupling in this system is dominated by thermal magnon-mediated scattering, suggesting fresh approaches to engineering device properties suitable for the desired applications.
Paper published in PRB in collaboration with Prof. Di Wu’s group
In collaboration with Prof. Di Wu’s group in our Department,We published a paper entitled “Enhanced spin accumulation in metallic bilayers with opposite spin Hall angles” in PRB [Physical Review B 99, 174406 (2019)].Spin accumulation can be generated via the spin Hall effect in a nonmagnetic material. It was previously found that spin accumulation and associated spintronic phenomena are attenuated in metallic bilayer with opposite spin angles. Here, we investigate the spin Hall magnetoresistance (SMR) in Pt/Y3Fe5O12 (YIG) with a thin W capping layer, in which W and Pt have opposite spin Hall angles. We find an increase of the SMR ratio with a W capping layer thinner than 1.0 nm. According to theoretical simulation, we attribute this phenomenon to the enhancement of the spin accumulation at the Pt/YIG interface, opposite to previous observations. Our findings provide a new approach for generating spin accumulation and associated pure spin current intensity for spintronic applications
Controlling the Spectral Characteristics of a Spin-Current Auto-Oscillator with an Electric Field
We published a paper entitled “Controlling the Spectral Characteristics of a Spin-Current Auto-Oscillator with an Electric Field” in PR APPLIED [Physical Review Applied 8, 021001 (2017)]. In this work, we demonstrated that the characteristic currents required for the excitation, the intensity and the spectral characteristics of the generated magnetic nano-oscillation can be tuned by the gate voltage, and the effect of electrostatic gating becomes enhanced in the strongly nonlinear oscillation regime. Electric-field modulation of the current-induced magnetization oscillations and spin waves demonstrated in this work can be utilized for frequency mixing, synchronization, and in logic gates in spin wave-based electronic (magnonic) devices.
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